posted on 2016-05-11, 00:00authored byJE Mates, IS Bayer, JM Palumbo, PJ Carroll, Constantine M. Megaridis
Rapid advances in modern electronics place ever-accelerating demands on innovation
towards more robust and versatile functional components. In the flexible electronics domain, novel material solutions often involve creative uses of common materials to reduce cost, while maintaining uncompromised performance. Here we combine a commercially available
paraffin wax–polyolefin thermoplastic blend (elastomer matrix binder) with bulk-produced
carbon nanofibres (charge percolation network for electron transport, and for imparting
nanoscale roughness) to fabricate adherent thin-film composite electrodes. The simple
wet-based process produces composite films capable of sustained ultra-high strain (500%)
with resilient electrical performance (resistances of the order of 101
–102 O sq 1). The composites are also designed to be superhydrophobic for long-term corrosion protection, even maintaining extreme liquid repellency at severe strain. Comprised of inexpensive
common materials applied in a single step, the present scalable approach eliminates
manufacturing obstacles for commercially viable wearable electronics, flexible power storage devices and corrosion-resistant circuits.
Funding
This material is based upon work supported in part by the US National Science Foundation
under grant CBET-1066426. The custom stretching fixtures and SEM stubs were
constructed by the UIC instrument shop, and all SEM measurements were made at the
UIC Research Resources Center. The Research Open Access Publishing (ROAAP) Fund
of the University of Illinois at Chicago provided financial support towards the open
access publishing fee for this article.