posted on 2018-06-18, 00:00authored byParijat Sengupta, Yu Wen, Junxia Shi
A semi-classical analysis of magneto-thermopower behaviour, namely, the \textit{Seebeck} and \textit{Nernst} effect (NE) in quantum wells of IV-VI lead salts with significant extrinsic Rashba spin-orbit coupling (RSOC) is performed in this report. In addition to the spin-dependent Seebeck effect that has been observed before, we also theoretically predict a similar spin-delineated behaviour for its thermal analog, the spin-dependent NE. The choice of lead salts follows from a two-fold advantage they offer, in part, to their superior thermoelectric properties, especially PbTe, while their low band gaps and high spin-orbit coupling make them ideal candidates to study \textit{RSOC} in nanostructures. The calculations show a larger longitudinal magneto-thermopower for the spin-up electrons while the transverse components are nearly identical. In contrast, for a magnetic field free case, the related power factor calculations reveal a significantly higher contribution from the spin-down ensemble and suffer a reduction with an increase in the electron density. We also discuss qualitatively the limitations of the semi-classical approach for the extreme case of a high magnetic field and allude to the observed thermopower behaviour when the quantum Hall regime is operational. Finally, techniques to modulate the thermopower are briefly outlined.
History
Citation
Sengupta, P., Wen, Y. and Shi, J. Spin-dependent magneto-thermopower of narrow-gap lead chalcogenide quantum wells. Scientific Reports. 2018. 8(1). 10.1038/s41598-018-23511-2. Article